World’s largest Span.-speaking nation by area

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Possible Answers:

ARG.

Last seen on: Wall Street Journal Crossword – June 25 2020 – It’s a Stretch

Random information on the term “ARG”:

Arg (Persian: ارگ‎, also Romanized as Ārg) is a village in Rizab Rural District, Qatruyeh District, Neyriz County, Fars Province, Iran. At the 2006 census, its population was 189, in 45 families.

ARG on Wikipedia